Disc/Cassette 1

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1.
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First Season Main Title (revised/extended) (01:00)
by Jerry Goldsmith - arranged by Morton Stevens
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2.
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Jerry Goldsmith Medley (02:57)
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3.
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The Quadripartite Affair (03:27)
by Walter Scharf
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4.
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The Double Affair, suite no. 2 (06:20)
by Morton Stevens
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5.
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Belly Laughs (02:21)
by Jerry Goldsmith
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6.
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The Finny Foot Affair (04:51)
by Morton Stevens
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7.
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The Fiddlesticks Affair, suite no. 2 (05:17)
by Lalo Schifrin
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8.
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The Yellow Scarf Affair (03:35)
by Morton Stevens
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9.
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Meet Mr. Solo (03:03)
by Jerry Goldsmith
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10.
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The Spy with my Face (04:09)
by Morton Stevens
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11.
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he Discotheque Affair, suite no. 2 (04:31)
by Gerald Fried
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12.
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The Nowhere Affair (02:48)
by The Nowhere Affair
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13.
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U.N.C.L.E. A Go Go (03:05)
by Gerald Fried
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14.
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The Bat Cave Affair (04:42)
by Gerald Fried
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15.
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One of our Spies is missing (01:09)
by Gerald Fried
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16.
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The Monks of St. Thomas Affair, suite no. 2 (03:46)
by Gerald Fried
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17.
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The Spy in the green Hat (03:19)
by Jerry Goldsmith - arranged by Gerald Fried & Robert Armbruster
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18.
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Gerald Fried Medley (07:21)
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19.
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The Karate Killers (01:51)
by Gerald Fried
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20.
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Richard Shores Medley (06:37)
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Disc/Cassette 2

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1.
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The Girl From U.N.C.L.E. Main Title (00:34)
by Jerry Goldsmith - arranged by David Grusin
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2.
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The Dog-gone Affair (05:28)
by David Grusin
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3.
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The Prisoner of Zalamar Affair (06:32)
by Richard Shores
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4.
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The Mother Muffin Affair (10:59)
by David Grusin
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5.
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The Mata Hari Affair (07:44)
by David Grusin
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6.
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The Montori Device Affair (05:31)
by Richard Shores
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7.
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The Horns-of-the-Dilemma Affair (02:05)
by Jack Marshall
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8.
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The Girl From U.N.C.L.E. End Title (00:39)
by Jerry Goldsmith - arranged by David Grusin
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9.
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The Deadly Quest Affair: Teaser (03:57)
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10.
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The Deadly Quest Affair: Act I (07:48)
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11.
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The Deadly Quest Affair: Act II (09:07)
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12.
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The Deadly Quest Affair: Act III (07:24)
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13.
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The Deadly Quest Affair: Act IV (08:06)
by Jerry Goldsmith
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